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Enable smtp.office365.com

535 5.7.3 Authentication unsuccessful
You need to set SmtpClientAuthenticationDisabled to false.

Connect to Office 365.

get-CASMailbox -Identity user@domain.com | fl SmtpClientAuthenticationDisabled
Set-CASMailbox -Identity user@domain.com -SmtpClientAuthenticationDisabled $false

Server: smtp.office365.com
Poort: 587
Versleuteling: STARTTLS